The Knights of Columbus have published the "Luke E. Hart Series", a collection of 30 pamphlets on various aspects of the Catholic faith, through their Catholic Information Service. But they've taken it a step further, in that they're producing podcasts of each of the pamphlets that will also be available through the CIS website, as well as through iTunes.
Check out a sampling of the podcast. They've even gotten a familiar Priest or two to be the voices of the podcasts.
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